Selective Metal-Phenolic Assembly from Complex Multicomponent Mixtures

G Lin; MA Rahim; MG Leeming; C Cortez-Jugo; QA Besford; Y Ju; QZ Zhong; ST Johnston; J Zhou; F Caruso

Journal article

Selective Metal-Phenolic Assembly from Complex Multicomponent Mixtures

G Lin, MA Rahim, MG Leeming, C Cortez-Jugo, QA Besford, Y Ju, QZ Zhong, ST Johnston, J Zhou, F Caruso

ACS Applied Materials and Interfaces | Published : 2019

DOI: 10.1021/acsami.9b04195

Download PDF

Abstract

Selective self-assembly in multicomponent mixtures offers a method for isolating desired components from complex systems for the rapid production of functional materials. Developing approaches capable of selective assembly of "target" components into intended three-dimensional structures is challenging because of the intrinsically high complexity of multicomponent systems. Herein, we report the selective coordination-driven self-assembly of metal-phenolic networks (MPNs) from a series of complex multicomponent systems (including crude plant extracts) into thin films via metal chelation with phenolic ligands. The metal (FeIII) selectively assembles low abundant phenolic components (e.g., myri..

View full abstract

University of Melbourne Researchers

Michael Leeming Author

Christina Cortez-Jugo Author

Yi David Ju Author

Stuart Johnston Author

Related Projects (3)

ARC CENTRE OF EXCELLENCE IN CONVERGENT BIO–NANO SCIENCE AND TECHNOLOGY

The CoE in Convergent Bio-Nano Science &Technology comprises a multi-disciplinary team focused on research aiming to understand and control ..

Engineering Multifunctional Particles for Biological Applications

This project aims to engineer multifunctional particles, examine their biological interactions and create particles for cell targeting, cell..

ADVANCING NANOMEDICINE THROUGH PARTICLE TECHNOLOGY

This proposal will support the development of advanced particle systems to improve the delivery of medicines in neurological diseases, HIV, ..

Grants

Awarded by Australian Research Council

Funding Acknowledgements

This research was conducted and funded by the Australian Research Council Centre (ARC) of Excellence in Convergent Bio-Nano Science and Technology (project number CE140100036) and an ARC Discovery Project (DP170103331). F.C. acknowledges the award a National Health and Medical Research Council Senior Principal Research Fellowship (APP1135806). This work was performed in part at the Materials Characterisation and Fabrication Platform (MCFP) at The University of Melbourne and the Victorian Node of the Australian National Fabrication Facility (ANFF). We also acknowledge Sergey Rubanov from the Bio21 Advanced Microscopy Facility (The University of Melbourne) for assistance with TEM.